By Frank Bolz (Auth.)
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Extra resources for Advanced Materials in Catalysis
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Yakubenok, E. , and Podvyazkin, Yu. A. (1974). Khim. Khim. Tekhnol. Polim. Org. Sint. 73, 29. Yates, D . J. C , and Sinfelt, J. H. (1967). J. Catal. 8, 348. Yates, D . J. C , and Sinfelt, J. H. (1969). J. Catal. 14, 182. 2 Physical and Chemical of Supported Bimetallic Properties Catalysts James J. Burton Robert L. Garten Exxon Research and Engineering Company Linden, New Jersey 1. 11. Introduction 33 T h e C h e m i c a l N a t u r e of B i m e t a l l i c C a t a l y s t s 35 A. Separate Metals or Bimetallic Clusters?
The Mössbauer parameters and dispersions of the bimetallic cata lysts given in Fig. 1 are listed in Table I, along with data for bulk P t F e and P d F e alloys. The isomer shift (δ) is the centroid of the Mössbauer spectrum and is determined by the s electron density at the Fe nucleus. Alteration of the nuclear s electron density results primarily from changes in the valence s electrons and the valence d electrons, the latter via changes in the screening of the s electrons. Examination of Table I shows that the isomer shift depends on the nature of the second metal in the bimetallic catalyst.
Advanced Materials in Catalysis by Frank Bolz (Auth.)